Increase of vaccines adjuvanticity by succinylation of vaccine antigen





A.V. Martynov, E.M. Babych, M.V. Smelyanskaya

Mechnicov institute of microbiology and immunology, 14-Puschinskaya St., Kharkov, 61057, Ukraine



Low adjuvanticity of vaccine antigens is one of the main problems in development of antiviral and anticancer vaccines. This situation forces researches to use a number of adjuvants. When Freundt adjuvant was used with diphtherial anatoxin (as vaccine antigen) maximum titer of induced antibodies was 1:500 at injection introducton of vaccine in accordance with Pasteur scheme. We have developed technology for increasing vaccine antigen adjuvanticity by 100 times at oral use of such antigen. Technology is based on partial chemical modification of vaccine protein antigen. Protein antigen was acylated by succinic anhydride by 3% (3 mg of succinic anhydride with 100 mg of protein, in accordance with scheme of professor D.K.F.Meijer). Oral introduction of such antigen to rabbits by Pasteur scheme (1, 3, 5, 9 and 12-th days by 5 mg of 1% solution) resulted in induction of protective antibodies against herpes simplex virus (strain L-2, C3hc4, Ring Domain) which had titer 1:5000. The induced antibodies protected test group of rabbits during 2 years. Peptide mapping of complexes viral antigen+antibody indicates the formation of antigens to absolutely new 'internal' epitopes of viral antigens. We guess that in animal intestine incomplete hydrolysis of modified antigen occurs to rather large peptides which are soaked up and induce high titers of antibodies. Similar results we obtained for diphtheria toxin (modification of 3% protein mass was followed by inactivation by formalin), Rhinovirus 14 protein (HRV14), Influenza Virus Hemagglutinin (2VIR). Now we obtained results which give hopes on testing chemically modified IE1 cytomegalovirus antigen. To decrease quantity of antigen and to check the incomplete hydrolysis hypothesis we changed the scheme of vaccine obtaining: after 3% acylation of IE1 structure the antigen obtained was treated by enzymes immobilized on sepharose (trypsin and papain) and then introduced by subcutaneous injection to rabbits (in dose 1 ml of 1% solution). In 2 weeks titer of protective antibodies in animal blood was 1:500. This fact indicates general rule: chemical modification by acylation of 3% protein mass results in a sharp increase of vaccine adjuvanicity that is caused by incomplete hydrolysis of protected antigen and appearance of new unique accessible epitopes in vaccine antigen. In our opinion, the use of similar methods will allow to create polyvalent vaccine against many viruses and microorganisms as well as to increase adjuvanicity of anticancer vaccines.




Key words: adjuvanicity, oral vaccines, succinylation, cytomegalovirus, herpes simplex virus, diphtheria toxin, rhinovirus







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